Ruthenium Catalyst Metathesis

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Astruc and Lloyd-Jones have discussed early work on elucidating this basic mechanism.

This basic series of steps can be used to design a variety of processes, such as: ring-closing metathesis (RCM) in which a diene substrate forms a cycloalkene plus an alkene; cross-metathesis (CM) in which two alkenes are used to prepare two new alkenes; ring-opening metathesis polymerisation (ROMP) where a cyclic alkene is used to prepare a polymer; and acyclic diene metathesis (ADMET) where a diene substrate is polymerised to form a poly(alkene) chain (Scheme 1(b)).

Subsequently, Percy and Hillier studied the initiation of GH2 using kinetic experiments and DFT calculations.

A mixture of dissociative and interchange mechanisms was proposed to operate, with the balance of these processes dependent on the pre-catalyst and substrate.


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